Carbon nano-materials are widely used as reinforcing materials for aluminum-based composites due to their excellent metallurgical properties. This study presents an approach for manufacturing Al/C composites utilizing a high energy ball milling and laser powder bed fusion (LPBF) process. We prepared Al/C60 and Al/MWCNT composites under 25 different conditions to observe their microstructure and mechanical property trends according to laser power and scan speed. The relative density of LPBFed composites increased as the energy density increased due to the oxide layer present on the aluminum surface and the high laser reflectance. It was found that, as the energy density increased, the increase in nanohardness and elastic modulus of the LPBFed composites was due to the high relative density. However, the high laser power condition of 179 W resulted in the softening of materials due to grain coarsening, resulting in a decrease in nanohardness and elastic modulus. Under the same laser conditions, the nanohardness of the LPBFed Al/2 vol.% MWCNT composites was approximately 0.5 GPa higher than that of the LPBFed Al/1 vol.% C60 composites, which is explained by the high relative density and grain refinement strengthening.